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题名: TMSI-Promoted Vinylogous Michael Addition of Siloxyfuran to 2-Substituted Chromones: A General Approach for the Total Synthesis of Chromanone Lactone Natural Products
作者: Liu, J; Li, ZC; Tong, P; Xie, ZX(谢志翔); Zhang, Y(张元); Li, Y(李瀛)
收录类别: SCIE ; EI ; MEDLINE ; BIOSIS
出版日期: 2015-02-06
刊名: Journal of Organic Chemistry
卷号: 80, 期号:3, 页码:1632-1643
英文摘要: A concise and facile synthetic protocol for the construction of the 2-gamma-lactone chromanone skeleton has been achieved through a TMSI-promoted diastereoselective vinylogous Michael addition of siloxyfuran to 2-substituted chromones. The applicability of this method is demonstrated through the rapid access to the total syntheses of (+/-)-microdiplodiasone, (+/-)-lachnone C, and (+/-)-gonytolides C and G.
作者部门: [Liu, Jie ; Li, Zhanchao ; Tong, Pei ; Xie, Zhixiang ; Zhang, Yuan ; Li, Ying] Lanzhou Univ, Coll Chem & Chem Engn, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China
通讯作者: Zhang, Y (reprint author), Lanzhou Univ, Coll Chem & Chem Engn, State Key Lab Appl Organ Chem, 222 Tianshui South Rd, Lanzhou 730000, Peoples R China.
学科分类: Chemistry
文章类型: Article
所属项目编号: National Natural Science Foundation of China [21272099, 21472078, 21102066] ; Fundamental Research Funds for the Central Universities [lzujbky-2013-48]
所属项目名称: 国家自然科学基金项目 ; 中央高校基本科研业务费专项资金
项目资助者: NSFC ; LZU
语种: 英语
DOI: 10.1021/jo502571r
ISSN号: 0022-3263
WOS记录号: WOS:000349934600035
EI记录号: 20150700533083
PM记录号: 25560746
BIOSIS记录号: BCI:BCI201500304813
IR记录号: BCI:BCI201500304813
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.lzu.edu.cn/handle/262010/126503
Appears in Collections:化学化工学院_期刊论文

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Recommended Citation:
Liu, J,Li, ZC,Tong, P,et al. TMSI-Promoted Vinylogous Michael Addition of Siloxyfuran to 2-Substituted Chromones: A General Approach for the Total Synthesis of Chromanone Lactone Natural Products[J]. JOURNAL OF ORGANIC CHEMISTRY,2015,80(3):1632-1643.
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