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兰州大学机构库  > 化学化工学院  > 期刊论文
题名: Catalytic Asymmetric Construction of -Quaternary Cyclopentanones and Its Application to the Syntheses of (-)-1,14-Herbertenediol and (-)-Aphanorphine
其他题名: Catalytic Asymmetric Construction of α-Quaternary Cyclopentanones and Its Application to the Syntheses of (-)-1,14-Herbertenediol and (-)-Aphanorphine
作者: Zhu, DY; Xu, MH; Tu, YQ(涂永强); Zhang, FM(张辅民); Wang, SH(王少华)
收录类别: SCIE ; EI ; PubMed
出版日期: 2015-10-26
刊名: CHEMISTRY-A EUROPEAN JOURNAL
卷号: 21, 期号:44, 页码:15502-15505
出版者: WILEY
出版地: WEINHEIM
英文摘要: A novel and efficient strategy to build -benzylic quaternary cyclopentanones with excellent enantioselectivities (up to 96%ee) and high yields (up to 99% yield) has been developed, and its application demonstrated by the first catalytic asymmetric total synthesis of (-)-1,14-herbertenediol and the formal synthesis of (-)-aphanorphine.
关键词: asymmetric synthesis ; enantioselectivity ; organocatalysis ; quaternary stereocenters ; sesquiterpenes
作者部门: [Zhu, Dao-Yong ; Xu, Ming-Hui ; Tu, Yong-Qiang ; Zhang, Fu-Min ; Wang, Shao-Hua] Lanzhou Univ, State Key Lab Appl Organ Chem, Tianjin, Peoples R China ; [Zhu, Dao-Yong ; Xu, Ming-Hui ; Tu, Yong-Qiang ; Zhang, Fu-Min ; Wang, Shao-Hua] Lanzhou Univ, Coll Chem & Chem Engn, Lanzhou & Collaborat Innovat Ctr Chem Sci & Engn, Tianjin, Peoples R China ; [Wang, Shao-Hua] Lanzhou Univ, Sch Pharm, Chengdu 610064, Peoples R China ; [Wang, Shao-Hua] Sichuan Univ, Key Lab Drug Targeting & Drug Delivery Syst, Minist Educ, Chengdu 610064, Peoples R China
通讯作者: Tu, YQ (reprint author), Lanzhou Univ, State Key Lab Appl Organ Chem, Tianjin, Peoples R China.
学科分类: Chemistry
文章类型: Article
所属项目编号: NSFC [21202073, 21290180, 21272097, 21372104, 21472077] ; "111" Program of MOE ; MOST [2012ZX 09201101-003] ; Fundamental Research Funds for the Central Universities [lzujbky-2014-k20, lzujbky-2015-k12] ; Opening Project of Key Laboratory of Drug Targeting and Drug Delivery System, Ministry of Education (Sichuan University)
所属项目名称: 国家自然科学基金项目 ; 国家科技重大专项 ; 高等学校学科创新引智计划(111计划) ; 中央高校基本科研业务费专项资金
项目资助者: NSFC ; MOST ; MOE ; SAFEA ; LZU
语种: 英语
DOI: 10.1002/chem.201502700
ISSN号: 0947-6539
WOS记录号: WOS:000363885400008
EI记录号: 20154401457557
PM记录号: 26387785
IR记录号: WOS:000363885400008
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内容类型: 期刊论文
URI标识: http://ir.lzu.edu.cn/handle/262010/180202
Appears in Collections:化学化工学院_期刊论文

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Recommended Citation:
Zhu, DY,Xu, MH,Tu, YQ,et al. Catalytic Asymmetric Construction of -Quaternary Cyclopentanones and Its Application to the Syntheses of (-)-1,14-Herbertenediol and (-)-Aphanorphine[J]. CHEMISTRY-A EUROPEAN JOURNAL,2015,21(44):15502-15505.
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