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兰州大学机构库  > 化学化工学院  > 期刊论文
题名: Palladium-Catalyzed Intermolecular Aryldifluoroalkylation of Alkynes
作者: He, YT; Wang, Q; Li, LH; Liu, XY(刘雪原); Xu, PF(许鹏飞); Liang, YM(梁永民)
收录类别: SCIE ; MEDLINE ; BIOSIS
出版日期: 2015-11-06
刊名: ORGANIC LETTERS
卷号: 17, 期号:21, 页码:5188-5191
英文摘要: A palladium-catalyzed aryldifluoroalkylation of alkynes with ethyl difluoroiodoacetate and arylboronic acids as reaction partners is described. The alkyne difunctionalization process provides various aryldifluoroalkylated products in one pot under mild reaction conditions. A wide range of alkynes and diverse arylboronic acids are compatible with these reaction conditions. High reaction efficiency and broad substrate scope are the notable features of this transformation. Preliminary mechanistic investigations indicate that a difluoroalkyl radical addition pathway is involved in this transformation.
作者部门: [He, Yu-Tao ; Wang, Qiang ; Li, Lian-Hua ; Liu, Xue-Yuan ; Xu, Peng-Fei ; Liang, Yong-Min] Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China ; [Liang, Yong-Min] Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China
通讯作者: Liang, YM (reprint author), Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China.
学科分类: Chemistry
文章类型: Article
所属项目编号: National Natural Science Foundation (NSF) [21272101, 21472074, 21472073] ; Fundamental Research Funds for the Central Universities [lzujbky-2014-243] ; "111" Project [J1103307] ; Program for Changjiang Scholars, and Innovative Research Team in University [IRT1138]
所属项目名称: 国家自然科学基金项目 ; 国家基础科学人才培养基金项目 ; 长江学者和创新团队发展计划 ; 中央高校基本科研业务费专项资金
项目资助者: NSFC ; MOE ; LZU
语种: 英语
DOI: 10.1021/acs.orglett.5b02512
ISSN号: 1523-7060
WOS记录号: WOS:000364434900011
PM记录号: 26461434
BIOSIS记录号: BCI:BCI201600080149
IR记录号: WOS:000364434900011
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内容类型: 期刊论文
URI标识: http://ir.lzu.edu.cn/handle/262010/180223
Appears in Collections:化学化工学院_期刊论文

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Recommended Citation:
He, YT,Wang, Q,Li, LH,et al. Palladium-Catalyzed Intermolecular Aryldifluoroalkylation of Alkynes[J]. ORGANIC LETTERS,2015,17(21):5188-5191.
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