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兰州大学机构库  > 化学化工学院  > 期刊论文
题名: A Triazole Organocatalyst with Spiropyrrolidine Framework and its Application to the Catalytic Asymmetric Addition of Nitromethane to alpha,beta-Unsaturated Aldehydes
作者: Liu, WX; Chen, SK; Tian, JM; Tu, YQ(涂永强); Wang, SH(王少华); Zhang, FM(张辅民)
收录类别: SCIE
出版日期: 2015-12-14
刊名: ADVANCED SYNTHESIS & CATALYSIS
卷号: 357, 期号:18, 页码:3831-3835
出版者: WILEY
出版地: WEINHEIM
英文摘要: A series of new water-compatible "spiropyrrolidine triazole" catalysts was designed and synthesized. The asymmetric Michael addition of nitromethane and alpha,beta-unsaturated aldehydes in an aqueous system was investigated to evaluate these new catalysts, and the resulting adducts were obtained with excellent enantioselectivity (up to 95.5% ee) and moderate to good yield (63-88%).
关键词: azaspiro skeleton ; Michael addition ; nitromethane ; organic catalysis ; 1,2,3-triazoles ; alpha,beta-unsaturated aldehydes
作者部门: [Liu, Wen-Xing ; Tu, Yong-Qiang] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China ; [Liu, Wen-Xing ; Chen, Si-Kai ; Tian, Jin-Miao ; Tu, Yong-Qiang ; Wang, Shao-Hua ; Zhang, Fu-Min] Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China ; [Liu, Wen-Xing ; Chen, Si-Kai ; Tian, Jin-Miao ; Tu, Yong-Qiang ; Wang, Shao-Hua ; Zhang, Fu-Min] Lanzhou Univ, Coll Chem & Chem Engn, Lanzhou 730000, Peoples R China
通讯作者: Tu, YQ (reprint author), Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
学科分类: Chemistry
文章类型: Article
所属项目编号: NSFC [21202073, 21290180, 21272097, 21372104, 21472077] ; "973" Program of MOST [2010CB833203] ; "111" Program of MOE ; MOST [2012ZX 09201101-003]
所属项目名称: 国家自然科学基金项目 ; 国家重点基础研究发展计划以及国家重大科学研究计划(973计划) ; 国家科技重大专项 ; 高等学校学科创新引智计划(111计划)
项目资助者: NSFC ; MOST ; MOE ; SAFEA
语种: 英语
DOI: 10.1002/adsc.201500582
ISSN号: 1615-4150
WOS记录号: WOS:000368342800007
IR记录号: WOS:000368342800007
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内容类型: 期刊论文
URI标识: http://ir.lzu.edu.cn/handle/262010/180261
Appears in Collections:化学化工学院_期刊论文

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Recommended Citation:
Liu, WX,Chen, SK,Tian, JM,et al. A Triazole Organocatalyst with Spiropyrrolidine Framework and its Application to the Catalytic Asymmetric Addition of Nitromethane to alpha,beta-Unsaturated Aldehydes[J]. ADVANCED SYNTHESIS & CATALYSIS,2015,357(18):3831-3835.
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