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题名: Concise To tal Synthesis of Isospongian Diterpenoid (+/-)-Polyrhaphin D
作者: Wang, ZM; Xing, ZM; Liu, L; Zhang, H; Zhong, ZL; Xie, XG; She, XG(厍学功)
收录类别: SCIE
出版日期: 2016-07-01
刊名: CHEMISTRYSELECT
卷号: 1, 期号:1-10, 页码:2225-2227
出版者: WILEY
出版地: WEINHEIM
英文摘要: The first total synthesis of isospongian diterpenoid (+/-)-polyrhaphin D has been accomplished in 9 steps with 19% overall yield starting from the Wieland-Miescher ketone derivative. The key features of our synthesis include a sequential reduc-tion/Michael addition/aldol condenzation to assemble the A ring and an intramolecular dehydrative cyclization/olefin isomerization reaction to install the gamma-butenolide D ring.
关键词: Natural product ; total synthesis ; Wieland-Miescher ketone ; Birch reduction ; aldol condenzation
作者部门: [Wang, Zemin ; Xing, Zhimin ; Liu, Lin ; Zhang, Hao ; Zhong, Zhuliang ; Xie, Xingang ; She, Xuegong] Lanzhou Univ, Dept Chem, State Key Lab Appl Organ Chem, 222 South Tianshui Rd, Lanzhou 730000, Peoples R China ; [She, Xuegong] Collaborat Innovat Ctr Chem Sci & Engn, Tianjin 300071, Peoples R China
通讯作者: Xie, XG (reprint author), Lanzhou Univ, Dept Chem, State Key Lab Appl Organ Chem, 222 South Tianshui Rd, Lanzhou 730000, Peoples R China.
学科分类: Chemistry
文章类型: Article
所属项目编号: NSFC [21472079] ; PCSIRT [IRT_15R28] ; FRFCU [lzujbky-2015-50, lzujbky-2016ct02]
所属项目名称: 国家自然科学基金项目 ; 长江学者和创新团队发展计划 ; 中央高校基本科研业务费专项资金
项目资助者: NSFC ; MOE ; LZU
语种: 英语
DOI: 10.1002/slct.201600635
ISSN号: 2365-6549
WOS记录号: WOS:000395417800022
IR记录号: WOS:000395417800022
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内容类型: 期刊论文
URI标识: http://ir.lzu.edu.cn/handle/262010/188991
Appears in Collections:化学化工学院_期刊论文

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Recommended Citation:
Wang, ZM,Xing, ZM,Liu, L,et al. Concise To tal Synthesis of Isospongian Diterpenoid (+/-)-Polyrhaphin D[J]. CHEMISTRYSELECT,2016,1(1-10):2225-2227.
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