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题名: Cobaloxime-catalyzed hydration of terminal alkynes without acidic promoters
作者: Hou, ST; Yang, HJ; Cheng, B; Zhai, HB; Li, Y
收录类别: SCIE
出版日期: 2017-06-28
刊名: CHEMICAL COMMUNICATIONS
卷号: 53, 期号:51
出版者: ROYAL SOC CHEMISTRY
出版地: CAMBRIDGE
英文摘要: Cobaloxime (Co(dmgBF(2))(2)center dot 2H(2)O), an inexpensive first-row transition-metal complex, catalyzed hydration of terminal alkynes gave the corresponding methyl ketones in good to excellent yields under neutral conditions (additional protic acids and silver salts are not required). A wide range of functional groups, such as allyl ether, benzyl ethers, carboxylic esters, imides, amides, nitro, and halogens, were tolerated. The mild reaction conditions together with the inexpensive feature and easy availability of the catalyst well address the current challenges in the field of alkyne hydration.
作者部门: [Hou, Shengtai ; Yang, Hongjian ; Cheng, Bin ; Zhai, Hongbin ; Li, Yun] Lanzhou Univ, Coll Chem & Chem Engn, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China ; [Li, Yun] Chinese Acad Sci, Shanghai Inst Organ Chem, State Key Lab Bioorgan & Nat Prod Chem, Shanghai 200032, Peoples R China ; [Zhai, Hongbin] Peking Univ, Sch Chem Biol & Biotechnol, Lab Chem Genom, Shenzhen Grad Sch, Shenzhen 518055, Peoples R China
通讯作者: Zhai, HB ; Li, Y (reprint author), Lanzhou Univ, Coll Chem & Chem Engn, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China. ; Li, Y (reprint author), Chinese Acad Sci, Shanghai Inst Organ Chem, State Key Lab Bioorgan & Nat Prod Chem, Shanghai 200032, Peoples R China. ; Zhai, HB (reprint author), Peking Univ, Sch Chem Biol & Biotechnol, Lab Chem Genom, Shenzhen Grad Sch, Shenzhen 518055, Peoples R China.
学科分类: Chemistry
文章类型: Article
所属项目编号: National Natural Science Foundation of China [21572089] ; Program for Changjiang Scholars and Innovative Research Team in University [PCSIRT: IRT_15R28] ; FRFCU [lzujbky-2016-52, lzujbky-2016-ct02]
所属项目名称: 国家自然科学基金项目 ; 长江学者和创新团队发展计划 ; 中央高校基本科研业务费专项资金
项目资助者: NSFC ; MOE ; LZU
语种: 英语
DOI: 10.1039/c7cc03919k
ISSN号: 1359-7345
WOS记录号: WOS:000404282900029
IR记录号: WOS:000404282900029
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内容类型: 期刊论文
URI标识: http://ir.lzu.edu.cn/handle/262010/190177
Appears in Collections:化学化工学院_期刊论文

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作者单位: 16CHEM

Recommended Citation:
Hou, ST,Yang, HJ,Cheng, B,et al. Cobaloxime-catalyzed hydration of terminal alkynes without acidic promoters[J]. CHEMICAL COMMUNICATIONS,2017,53(51).
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