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题名: One-Pot Multicomponent Mechanosynthesis of Polysubstituted trans-2,3-Dihydropyrroles and Pyrroles from Amines, Alkyne Esters, and Chalcones
作者: Xu, H; Liu, HW; Chen, K; Wang, GW
收录类别: SCIE ; PUBMED
出版日期: 2018-06-01
刊名: JOURNAL OF ORGANIC CHEMISTRY
卷号: 83, 期号:1, 页码:6035-6049
出版者: AMER CHEMICAL SOC
出版地: WASHINGTON
英文摘要: An efficient and practical one-pot multicomponent reaction of amines with alkyne esters and chalcones promoted by I-2/PhI(OAc)(2) has been developed under solvent-free ball-milling conditions to afford a variety of polysubstituted trans-2,3-dihydropyrroles in moderate to good yields. The present method features a short reaction time, mild reaction conditions, broad substrate scope, and feasibility of large-scale synthesis. Intriguingly, this protocol can also furnish the corresponding synthetically more attractive pyrroles with the addition of an oxidant in a one-pot way.
作者部门: [Xu, Hui ; Liu, Hong-Wei ; Chen, Kuan ; Wang, Guan-Wu] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, iChEM Collaborat Innovat Ctr Chem Energy Mat, CAS Key Lab Soft Matter Chem, Hefei 230026, Anhui, Peoples R China ; [Xu, Hui ; Liu, Hong-Wei ; Chen, Kuan ; Wang, Guan-Wu] Univ Sci & Technol China, Dept Chem, Hefei 230026, Anhui, Peoples R China ; [Wang, Guan-Wu] Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Gansu, Peoples R China
通讯作者: Wang, GW (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, iChEM Collaborat Innovat Ctr Chem Energy Mat, CAS Key Lab Soft Matter Chem, Hefei 230026, Anhui, Peoples R China. ; Wang, GW (reprint author), Univ Sci & Technol China, Dept Chem, Hefei 230026, Anhui, Peoples R China. ; Wang, GW (reprint author), Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Gansu, Peoples R China.
学科分类: Chemistry
文章类型: Article
所属项目编号: National Natural Science Foundation of China [21372211] ; Strategic Priority Research Program of the Chinese Academy of Sciences [XDB20000000]
所属项目名称: 国家自然科学基金项目
项目资助者: NSFC
语种: 英语
DOI: 10.1021/acs.joc.8b00665
ISSN号: 0022-3263
WOS记录号: WOS:000434367700015
PM记录号: 29745226
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内容类型: 期刊论文
URI标识: http://ir.lzu.edu.cn/handle/262010/196912
Appears in Collections:化学化工学院_期刊论文

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Recommended Citation:
Xu, H,Liu, HW,Chen, K,et al. One-Pot Multicomponent Mechanosynthesis of Polysubstituted trans-2,3-Dihydropyrroles and Pyrroles from Amines, Alkyne Esters, and Chalcones[J]. JOURNAL OF ORGANIC CHEMISTRY,2018,83(1):6035-6049.
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