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兰州大学机构库  > 化学化工学院  > 期刊论文
题名: Ruthenium-Catalyzed Direct C-H Amidation of Arenes: A Mechanistic Study
作者: Zhang, LL; Li, LH; Wang, YQ; Yang, YF; Liu, XY(刘雪原); Liang, YM(梁永民)
收录类别: SCIE ; EI
出版日期: 2014-04-28
刊名: ORGANOMETALLICS
卷号: 33, 期号:8
出版者: AMER CHEMICAL SOC
出版地: WASHINGTON
英文摘要: We report mechanistic studies of C H activitation/amidation reactions using azides as the amino source catalyzed by [RuCl2(p-cymene)](2). We have achieved two intermediates in the catalytic cycle (C5H4NC6H4)Ru(p-cymene)Cl and (C5H4NC6H4)NArRu(p-cymene)Cl (Ar = NO2C6H4SO2). Furthermore, the process from (C5H4NC6H4)Ru(p-cymene)Cl to (C5H4NC6H4)NArRu(p-cymene)Cl was monitored by F-19 NMR and a ruthenium imido species was proposed to explain the formation of the azacyclopropane analogue.
作者部门: [Zhang, Lu-Lu ; Li, Lian-Hua ; Wang, Yu-Qi ; Yang, Yan-Fang ; Liu, Xue-Yuan ; Liang, Yong-Min] Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China
通讯作者: Liang, YM (reprint author), Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China.
学科分类: Chemistry
文章类型: Article
所属项目编号: National Science Foundation [NSF21072081] ; National Basic Research Program of China (973 Program) [2010CB8-33203] ; "111" Project ; Program for Changjiang Scholars and innovative Research Team in University [IRT1138]
所属项目名称: 国家自然科学基金项目 ; 国家重点基础研究发展计划以及国家重大科学研究计划(973计划) ; 长江学者和创新团队发展计划
项目资助者: NSFC ; MOST ; MOE
语种: 英语
DOI: 10.1021/om500080z
ISSN号: 0276-7333
WOS记录号: WOS:000335201600002
EI记录号: 20141917693836
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内容类型: 期刊论文
URI标识: http://ir.lzu.edu.cn/handle/262010/75398
Appears in Collections:化学化工学院_期刊论文

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Zhang, LL; Li, LH; Wang, YQ; Yang, YF; Liu, XY; Liang, YM.Ruthenium-Catalyzed Direct C-H Amidation of Arenes: A Mechanistic Study,ORGANOMETALLICS,2014,33(8):
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