兰州大学机构库 >化学化工学院
Ruthenium-Catalyzed Direct C-H Amidation of Arenes: A Mechanistic Study
Zhang, LL; Li, LH; Wang, YQ; Yang, YF; Liu, XY(刘雪原); Liang, YM(梁永民); Liang, YM (reprint author), Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China.
2014-04-28
发表期刊ORGANOMETALLICS
ISSN0276-7333
卷号33期号:8
出版者AMER CHEMICAL SOC
摘要We report mechanistic studies of C H activitation/amidation reactions using azides as the amino source catalyzed by [RuCl2(p-cymene)](2). We have achieved two intermediates in the catalytic cycle (C5H4NC6H4)Ru(p-cymene)Cl and (C5H4NC6H4)NArRu(p-cymene)Cl (Ar = NO2C6H4SO2). Furthermore, the process from (C5H4NC6H4)Ru(p-cymene)Cl to (C5H4NC6H4)NArRu(p-cymene)Cl was monitored by F-19 NMR and a ruthenium imido species was proposed to explain the formation of the azacyclopropane analogue.
出版地WASHINGTON
学科领域Chemistry
作者部门[Zhang, Lu-Lu;
Li, Lian-Hua;
Wang, Yu-Qi;
Yang, Yan-Fang;
Liu, Xue-Yuan;
Liang, Yong-Min] Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China
DOI10.1021/om500080z
文章类型Article
收录类别SCIE ; EI
所属项目编号National Science Foundation [NSF21072081] ; National Basic Research Program of China (973 Program) [2010CB8-33203] ; "111" Project ; Program for Changjiang Scholars and innovative Research Team in University [IRT1138]
语种英语
资助项目国家自然科学基金项目 ; 国家重点基础研究发展计划以及国家重大科学研究计划(973计划) ; 长江学者和创新团队发展计划
项目资助者National Science Foundation [NSF21072081]; National Basic Research Program of China (973 Program) [2010CB8-33203]; "111" Project; Program for Changjiang Scholars and innovative Research Team in University [IRT1138] ; NSFC ; MOST ; MOE
WOS记录号WOS:000335201600002
EI记录号20141917693836
第一机构
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文献类型期刊论文
条目标识符http://ir.lzu.edu.cn/handle/262010/75398
Collection化学化工学院
通讯作者Liang, YM (reprint author), Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China.
Recommended Citation:
GB/T 7714
Zhang, LL,Li, LH,Wang, YQ,et al. Ruthenium-Catalyzed Direct C-H Amidation of Arenes: A Mechanistic Study[J]. ORGANOMETALLICS,2014,33(8).
APA Zhang, LL.,Li, LH.,Wang, YQ.,Yang, YF.,Liu, XY.,...&Liang, YM .(2014).Ruthenium-Catalyzed Direct C-H Amidation of Arenes: A Mechanistic Study.ORGANOMETALLICS,33(8).
MLA Zhang, LL,et al."Ruthenium-Catalyzed Direct C-H Amidation of Arenes: A Mechanistic Study".ORGANOMETALLICS 33.8(2014).
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