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兰州大学机构库  > 化学化工学院  > 期刊论文
题名: Construction of Covalent Organic Framework for Catalysis: Pd/COF-LZU1 in Suzuki-Miyaura Coupling Reaction
作者: Ding, SY(丁三元); Gao, J; Wang, Q; Zhang, Y; Song, WG; Su, CY; Wang, W(王为)
收录类别: SCIE ; EI ; PubMed ; ESI
ESI注释: 2017-07-19;Highly Cited Papers
出版日期: 2011-12-14
刊名: JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷号: 133, 期号:49
出版者: AMER CHEMICAL SOC
出版地: WASHINGTON
英文摘要: Covalent organic frameworks (COFs) are crystalline porous solids with well-defined two- or three-dimensional molecular structures. Although the structural regularity provides this new type of porous material with high potentials in catalysis, no example has been presented so far. Herein, we report the first application of a new COF material, COF-LZU1, for highly efficient catalysis. The easily prepared imine-linked COF-LZU1 possesses a two-dimensional eclipsed layered-sheet structure, making its incorporation with metal ions feasible. Via a simple post-treatment, a Pd(II)-containing COF, Pd/COF-LZU1, was accordingly synthesized, which showed excellent catalytic activity in catalyzing the Suzuki-Miyaura coupling reaction. The superior utility of Pd/COF-LZU1 in catalysis was elucidated by the broad scope of the reactants and the excellent yields (96-98%) of the reaction products, together with the high stability and easy recyclability of the catalyst. We expect that our approach will further boost research on designing and employing functional COF materials for catalysis.
作者部门: [Ding, San-Yuan ; Gao, Jia ; Wang, Qiong ; Zhang, Yuan ; Wang, Wei] Lanzhou Univ, State Key Lab Appl Organ Chem, Coll Chem & Chem Engn, Lanzhou 730000, Gansu, Peoples R China ; [Wang, Qiong ; Song, Wei-Guo] Chinese Acad Sci, Inst Chem, Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China ; [Wang, Qiong ; Song, Wei-Guo] Chinese Acad Sci, Beijing Natl Lab Mol Sci BNLMS, Beijing 100190, Peoples R China ; [Su, Cheng-Yong] Sun Yat Sen Univ, Sch Chem & Chem Engn, Guangzhou 510275, Guangdong, Peoples R China
通讯作者: Wang, W (reprint author), Lanzhou Univ, State Key Lab Appl Organ Chem, Coll Chem & Chem Engn, Lanzhou 730000, Gansu, Peoples R China.
学科分类: Chemistry
文章类型: Article
所属项目编号: National Natural Science Foundation of China [20933009, 20972064] ; Chinese Ministry of Education [309028] ; 111 Project
所属项目名称: 国家自然科学基金项目 ; 教育部科学技术研究重大项目 ; 高等学校学科创新引智计划(111计划)
项目资助者: NSFC ; SAFEA ; MOE
语种: 英语
DOI: 10.1021/ja206846p
ISSN号: 0002-7863
WOS记录号: WOS:000298719800048
EI记录号: 20115014597783
PM记录号: 22026454
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内容类型: 期刊论文
URI标识: http://ir.lzu.edu.cn/handle/262010/76261
Appears in Collections:化学化工学院_期刊论文

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Recommended Citation:
Ding, SY; Gao, J; Wang, Q; Zhang, Y; Song, WG; Su, CY; Wang, W.Construction of Covalent Organic Framework for Catalysis: Pd/COF-LZU1 in Suzuki-Miyaura Coupling Reaction,JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2011,133(49):
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