兰州大学机构库
Atomically dispersed cobalt-nitrogen-carbon catalysts for efficient oxidative esterification of aromatic alcohols
Zhang, Fengwei1; Liu, Peihao1; Li, Jingjing1; Guo, Hefang1; Zhang, Han1; Zhang, Zehui3; Dong, Zhengping2
2023-08-14
Online publication date2023-07
Source PublicationNEW JOURNAL OF CHEMISTRY   Impact Factor & Quartile
ISSN1144-0546 ; 1369-9261
Volume47Issue:32Pages:15036-15046
page numbers11
AbstractDesigning and synthesizing highly efficient non-noble metal-based catalysts with uniform active sites provide a powerful platform for recognizing real active sites and understanding catalytic reaction mechanisms. Herein, we prepared a series of N-doped graphene-like carbon (NG) intercalated Co-based single/dual-atom catalysts via a hard template-assisted spatial confinement strategy. Comprehensive characterization studies confirmed the atomically dispersed cobalt single atom active sites. The obtained Co SACs@NG-800-50 catalyst exhibits satisfying activity and selectivity for oxidative esterification of benzyl alcohol and other investigated alcohols under mild conditions. The catalyst can effectively activate O-2 to generate O2- active species through abundant CoN3 active sites, thus promoting the smooth progress of oxidative esterification of aromatic alcohols. Moreover, the catalyst displays excellent structural stability and recycling durability even after 6 reactions.
PublisherROYAL SOC CHEMISTRY
DOI10.1039/d3nj02558f
Indexed BySCIE
Language英语
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:001034053900001
Original Document TypeArticle
Citation statistics
Document Type期刊论文
Identifierhttps://ir.lzu.edu.cn/handle/262010/568889
Collection兰州大学
Corresponding AuthorZhang, Fengwei; Zhang, Zehui; Dong, Zhengping
Affiliation
1.Shanxi Univ, Inst Crystalline Mat, Inst Mol Sci, Taiyuan 030006, Peoples R China;
2.Lanzhou Univ, Coll Chem & Chem Engn, Lanzhou 730000, Peoples R China;
3.South Cent Univ Nationalities, Key Lab Catalysis & Mat Sci, Minist Educ, Wuhan 430074, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Fengwei,Liu, Peihao,Li, Jingjing,et al. Atomically dispersed cobalt-nitrogen-carbon catalysts for efficient oxidative esterification of aromatic alcohols[J]. NEW JOURNAL OF CHEMISTRY,2023,47(32):15036-15046.
APA Zhang, Fengwei.,Liu, Peihao.,Li, Jingjing.,Guo, Hefang.,Zhang, Han.,...&Dong, Zhengping.(2023).Atomically dispersed cobalt-nitrogen-carbon catalysts for efficient oxidative esterification of aromatic alcohols.NEW JOURNAL OF CHEMISTRY,47(32),15036-15046.
MLA Zhang, Fengwei,et al."Atomically dispersed cobalt-nitrogen-carbon catalysts for efficient oxidative esterification of aromatic alcohols".NEW JOURNAL OF CHEMISTRY 47.32(2023):15036-15046.
Files in This Item:
There are no files associated with this item.
Related Services
Recommend this item
Bookmark
Usage statistics
Export to Endnote
Altmetrics Score
Google Scholar
Similar articles in Google Scholar
[Zhang, Fengwei]'s Articles
[Liu, Peihao]'s Articles
[Li, Jingjing]'s Articles
Baidu academic
Similar articles in Baidu academic
[Zhang, Fengwei]'s Articles
[Liu, Peihao]'s Articles
[Li, Jingjing]'s Articles
Bing Scholar
Similar articles in Bing Scholar
[Zhang, Fengwei]'s Articles
[Liu, Peihao]'s Articles
[Li, Jingjing]'s Articles
Terms of Use
No data!
Social Bookmark/Share
No comment.
Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.